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Synthesis of Biotinylated 2-Methoxystypandrone and Identification of Jak2 and Ikk as Its Targets
SUNLONG BIOTECH / 2024-01-09
  • Author:Kuang, S., Sima, Z., Liu, J., Li, W., Song, Q., Zhang, Q. & Yu, Q.

  • Periodical:Anti-cancer agents in medicinal chemistry 18, 422-427 (2018)

  • Article source

BACKGROUND: 2-Methoxystypandrone (2-MS), isolated from the roots of Polygonum cuspidatum, is a potent dual inhibitor of the STAT3 and NF-κB pathways. OBJECTIVE: To investigate the molecular targets and mechanisms of 2-MS. METHOD: A biotin-conjugated 2-MS analog, named 2-MS-Biotin, was designed and synthesized. The effects of 2-MS-Biotin on the STAT3 and NF-κB pathways were examined by Western blotting. The cytotoxicity of 2- MS-Biotin was evaluated using real-time cell analysis system. Proteins directly bound to 2-MS-Biotin were pulled down through streptavidin agarose beads and were detected using Western blotting. RESULTS: 2-MS-Biotin retained the inhibition activities of the parent compound 2-MS on the STAT3 and NF-κB pathways as well as on cancer cell growth. Also, JAK2 and IKK proteins can be effectively pulled down by 2- MS-Biotin. CONCLUSION: Using 2-MS-Biotin as a tool, both JAK2 and IKK were identified as the targets of 2-MS.

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